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Ultra-sensitive polarization-resolved black phosphorus homojunction photodetector defined by ferroelectric domains

Shuaiqin Wu, Yan Chen, Xudong Wang, Hanxue Jiao, Qianru Zhao, Xinning Huang, Xiaochi Tai, Yong Zhou, Hao Chen, Xingjun Wang, Shenyang Huang, Hugen Yan, Tie Lin, Hong Shen, Weida Hu, Xiangjian Meng, Junhao Chu, Jianlu Wang

Nature Communications · 2022

Research context

Abstract With the further miniaturization and integration of multi-dimensional optical information detection devices, polarization-sensitive photodetectors based on anisotropic low-dimension materials have attractive potential applications. However, the performance of these devices is restricted by intrinsic property of materials leading to a small polarization ratio of the detectors. Here, we construct a black phosphorus (BP) homojunction photodetector defined by ferroelectric domains with ultra-sensitive polarization photoresponse. With the modulation of ferroelectric field, the BP exhibits anisotropic dispersion changes, leading an increased photothermalelectric (PTE) current in the armchair (AC) direction. Moreover, the PN junction can promote the PTE current and accelerate carrier separation. As a result, the BP photodetector demonstrates an ultrahigh polarization ratio (PR) of 288 at 1450 nm incident light, a large photoresponsivity of 1.06 A/W, and a high detectivity of 1.27 × 10 11 cmHz 1/2 W −1 at room temperature. This work reveals the great potential of BP in future polarized light detection.

Keywords: Photodetector, Homojunction, Optoelectronics, Ferroelectricity, Materials science, Polarization (electrochemistry), Specific detectivity, Responsivity, Optics, Physics, Doping, Dielectric, Chemistry, Physical chemistry

Source & review

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Retained from the existing reviewed corpus.

237 citations · OpenAlex · observed 2026-09-08

Metadata: OpenAlex, existing-corpus · source record ↗

device

ferroelectric-domain-defined black phosphorus homojunction photodetector

Source PDF · page 1
material

black phosphorus

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mechanism

photothermoelectric contribution in the detector

Source PDF · page 3
metric

polarization ratio 288 at 1450 nm

Source PDF · page 1

Cite / 引用

Shuaiqin Wu, Yan Chen, Xudong Wang, Hanxue Jiao, Qianru Zhao, Xinning Huang, Xiaochi Tai, Yong Zhou, Hao Chen, Xingjun Wang, Shenyang Huang, Hugen Yan, Tie Lin, Hong Shen, Weida Hu, Xiangjian Meng, Junhao Chu, Jianlu Wang. Ultra-sensitive polarization-resolved black phosphorus homojunction photodetector defined by ferroelectric domains. Nature Communications (2022). https://doi.org/10.1038/s41467-022-30951-y

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