E IN PRESS ARTICLE IN PRESS Abstract As a type of promising hardware for next-generation artificial visual systems with extended perceptual and anti-interference capabilities, circular-polarization-resolved retinomorphic sensors are underexplored due to the lack of suitable chiral materials that enable highly dissymmetric circular-polarization responses and multiple biomimetic functions. Here, we demonstrate a self- assembly heterogeneous microstructure consisting of chiral-deficient grains and chiral-rich grain boundaries in chiral perovskites that simultaneously facilitate spin selectivity and optoelectronic properties for highly dissymmetric and multifunctional circular-polarization-resolved retinomorphic sensors. Our sensors not only exhibit a photocurrent dissymmetry factor as high as 1.98 and a panchromatic circular-polarization-resolved response, but also possess multiple biomimetic functions that simulate human retinas, including synaptic behaviors, light adaptation, and color recognition. As a proof-of-concept, we respectively demonstrate their applications using a sensor array that resolves a single circular-polarization handedness for information encry
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Spin-selective heterogeneous chiral perovskites for circular-polarization-resolved retinomorphic sensors
De Yu, Xin Zhang, Tao Wang, Yuheng Li, Ruiqin He, Zeyang Xu, Jixin Tang, Yixuan Zhang, Xinmiao Zhang, Huang Huang, Tongpeng Zhao, Haoliang Liu, Ao Liu, Kai Shen, Sai Bai, Huihui Zhu, Yimu Chen, Qinghai Song
Research context
As a type of promising hardware for next-generation artificial visual systems with extended perceptual and anti-interference capabilities, circular-polarization-resolved retinomorphic sensors are underexplored due to the lack of suitable chiral materials that enable highly dissymmetric circular-polarization responses and multiple biomimetic functions. Here, we demonstrate a self-assembly heterogeneous microstructure consisting of chiral-deficient grains and chiral-rich grain boundaries in chiral perovskites that simultaneously facilitate spin selectivity and optoelectronic properties for highly dissymmetric and multifunctional circular-polarization-resolved retinomorphic sensors. Our sensors not only exhibit a photocurrent dissymmetry factor as high as 1.98 and a panchromatic circular-polarization-resolved response, but also possess multiple biomimetic functions that simulate human retinas, including synaptic behaviors, light adaptation, and color recognition. As a proof-of-concept, we respectively demonstrate their applications using a sensor array that resolves a single circular-polarization handedness for information encryption, as well as binocular sensor arrays that resolve th
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De Yu, Xin Zhang, Tao Wang, Yuheng Li, Ruiqin He, Zeyang Xu, Jixin Tang, Yixuan Zhang, Xinmiao Zhang, Huang Huang, Tongpeng Zhao, Haoliang Liu, Ao Liu, Kai Shen, Sai Bai, Huihui Zhu, Yimu Chen, Qinghai Song. Spin-selective heterogeneous chiral perovskites for circular-polarization-resolved retinomorphic sensors. Nature Communications (2026). https://doi.org/10.1038/s41467-026-71190-9
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